Polymeric Composites and Foams based on Two Dimensional Surfactants

Project Personnel

Douglas Adamson

Principal Investigator

University of Connecticut

Email

Andrey Dobrynin

University of Akron

Email

Hannes Schniepp

College of William and Mary

Email

Funding Divisions

Division of Materials Research (DMR), Civil, Mechanical and Manufacturing Innovation (CMMI)

The challenge of mixing different materials such as plastics, particles, and solvents is one of the major factors hindering future advances in the development of functional materials with new or improved properties. A prominent example of this are graphene-based materials, where graphene's extraordinary combination of high strength, surface area, and conductivity cannot yet be fully utilized as graphene sheets tend to clump together and stack due to a lack of compatibility with other materials. Boron nitride sheets are another example of a promising material limited by the same problem. This project attempts to overcome this obstacle by utilizing the high-energy interface between two immiscible solvents to force stacked graphene sheets to exfoliate and spread. The understanding of governing physical principles of surface activity of graphene and boron nitride produced by this activity will be applied to form emulsions that serve as precursors for the synthesis of foam-like materials reinforced with graphene or boron nitride with optimized mechanical and electrical properties. These reinforced polymeric materials have the potential to be used as strong and lightweight structural materials, electrodes in capacitors and batteries, substrates for flexible electronics, electrically conductive, high surface area catalyst supports, and super-absorbent materials. The project will also be of societal benefit as a result of outreach activities built on the Chemistry Wizards Program designed to target middle school children learning about scientific inquiry. The program aims to spur students from underrepresented populations to pursue post-secondary study and careers in STEM fields.

Publications

Evolution of Heterogeneity and Chemical Functionality during the Oxidation of Graphite
H. V. Kumar, A. J. Oyer, K. Y. -. Huang, and D. H. Adamson
8/29/2022
Ultra‐Tough Elastomers from Stereochemistry‐Directed Hydrogen Bonding in Isosorbide‐Based Polymers
S. R. Petersen, H. Prydderch, J. C. Worch, C. J. Stubbs, Z. Wang, J. Yu, M. C. Arno, A. V. Dobrynin, M. L. Becker, and A. P. Dove
3/4/2022
Chromatographic Approach to Isolate Exfoliated Graphene
P. G. Abeykoon, S. P. Ward, F. Chen, and D. H. Adamson
7/29/2021
Boron Nitride Nanotube Impurity Detection and Purity Verification
M. S. Amin, T. E. Molin, C. Tampubolon, D. E. Kranbuehl, and H. C. Schniepp
10/29/2020
Interface-exfoliated graphene-based conductive screen-printing inks: low-loading, low-cost, and additive-free
F. Chen, D. Varghese, S. T. McDermott, I. George, L. Geng, and D. H. Adamson
10/22/2020
Effect of Aqueous Anions on Graphene Exfoliation
S. P. Ward, P. G. Abeykoon, S. T. McDermott, and D. H. Adamson
8/14/2020
Self-Assembled Graphene Composites for Flow-Through Filtration
D. Varghese, J. L. Bento, S. P. Ward, and D. H. Adamson
6/16/2020
Tissue-Mimetic Dielectric Actuators: Free-Standing, Stable, and Solvent-Free
V. Karimkhani, M. Vatankhah-Varnosfaderani, A. N. Keith, E. Dashtimoghadam, B. J. Morgan, M. Jacobs, A. V. Dobrynin, and S. S. Sheiko
4/1/2020
Advanced Manufacturing for Biomaterials and Biological Materials, Part II
S. E. Naleway, V. Thomas, D. Restrepo, and H. C. Schniepp
2/14/2020
Advanced Manufacturing for Biomaterials and Biological Materials, Part I
D. Restrepo, S. E. Naleway, V. Thomas, and H. C. Schniepp
1/22/2020
Using atomic force spectroscopy to study oil/mineral interactions at reservoir temperatures and pressures
W. W. Dickinson, S. S. J. Aravind, S. R. Higgins, S. Berg, B. M. J. M. Suijkerbuijk, and H. C. Schniepp
1/1/2020
Characterization of graphene oxide: Variations in reported approaches
Z. Zhang, H. C. Schniepp, and D. H. Adamson
12/1/2019
Pristine Graphene Microspheres by the Spreading and Trapping of Graphene at an Interface
C. D. Liyanage, D. Varghese, E. E. B. Brown, and D. H. Adamson
10/24/2019
High-Purity Boron Nitride Nanotubes via High-Yield Hydrocarbon Solvent Processing
M. S. Amin, B. Atwater, R. D. Pike, K. E. Williamson, D. E. Kranbuehl, and H. C. Schniepp
10/11/2019
Brush-Like Polymers and Entanglements: From Linear Chains to Filaments
H. Liang, G. S. Grest, and A. V. Dobrynin
9/26/2019
Electrical Conductivity of Graphene–Polymer Composite Foams: A Computational Study
Z. Wang, Y. Tian, H. Liang, D. H. Adamson, and A. V. Dobrynin
9/25/2019
Nonlinear Elasticity and Swelling of Comb and Bottlebrush Networks
M. Jacobs, H. Liang, E. Dashtimoghadam, B. J. Morgan, S. S. Sheiko, and A. V. Dobrynin
6/28/2019
Polymer crystallinity and the ductile to brittle transition
S. J. A. Hocker, W. T. Kim, H. C. Schniepp, and D. E. Kranbuehl
12/1/2018
High-throughput optical thickness and size characterization of 2D materials
W. W. Dickinson, H. V. Kumar, D. H. Adamson, and H. C. Schniepp
1/1/2018
Graphene oxide reduces the hydrolytic degradation in polyamide-11
S. J. A. Hocker, N. V. Hudson-Smith, P. T. Smith, C. H. Komatsu, L. R. Dickinson, H. C. Schniepp, and D. E. Kranbuehl
9/1/2017
Altering and investigating the surfactant properties of graphene oxide
H. V. Kumar, K. Y. -. Huang, S. P. Ward, and D. H. Adamson
5/1/2017
Controlled 3D Assembly of Graphene Sheets to Build Conductive, Chemically Selective and Shape‐Responsive Materials
S. J. Woltornist, D. Varghese, D. Massucci, Z. Cao, A. V. Dobrynin, and D. H. Adamson
3/6/2017
Thermal and Electrical Properties of Nanocomposites Based on Self‐Assembled Pristine Graphene
J. L. Bento, E. Brown, S. J. Woltornist, and D. H. Adamson
11/23/2016
Atomic Force Spectroscopy Using Colloidal Tips Functionalized with Dried Crude Oil: A Versatile Tool to Investigate Oil–Mineral Interactions
L. R. Dickinson, B. M. J. M. Suijkerbuijk, S. Berg, F. H. M. Marcelis, and H. C. Schniepp
10/27/2016
Assessing graphene oxide/polymer interfacial interactions by way of peeling test
L. R. Dickinson, D. E. Kranbuehl, and H. C. Schniepp
9/1/2016
Enhancing polyimide's water barrier properties through addition of functionalized graphene oxide
S. Hocker, N. Hudson-Smith, H. C. Schniepp, and D. E. Kranbuehl
6/1/2016
AFM-based mechanical characterization of single nanofibres
B. R. Neugirg, S. R. Koebley, H. C. Schniepp, and A. Fery
1/1/2016

View All Publications

Research Highlights

Polymer Foams for Oil Recovery
Douglas Adamson
11/3/2022
Controlled 3D Assembly of Graphene Sheets
Andrey Dobrynin and Douglas Adamson
3/6/2017

Designing Materials to Revolutionize and Engineer our Future (DMREF)